Article

Giant electron phonon coupling of the breathing plane oxygen phonons in the dynamic stripe phase of La1.67Sr0.33NiO4

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https://scholar.colorado.edu/concern/articles/1g05fc847
Abstract
  • (LSNO) is a classic example of such a material. At low temperatures holes introduced via substitution of La by Sr segregate into lines to form boundaries between magnetically ordered domains in the form of stripes. The stripes become dynamic at high temperatures, but LSNO remains insulating presumably because an interplay between magnetic correlations and electron–phonon coupling localizes charge carriers. Magnetic degrees of freedom have been extensively investigated in this system, but phonons are almost completely unexplored. We searched for electron–phonon anomalies in LSNO by inelastic neutron scattering. Giant renormalization of plane Ni–O bond-stretching modes that modulate the volume around Ni appears on entering the dynamic charge stripe phase. Other phonons are a lot less sensitive to stripe melting. Dramatic overdamping of the breathing modes indicates that dynamic stripe phase may host small polarons. We argue that this feature sets electron–phonon coupling in nickelates apart from that in cuprates where breathing phonons are not overdamped and point out remarkable similarities with the colossal magnetoresistance manganites.

Creator
Date Issued
  • 2020
Academic Affiliation
Journal Title
Journal Issue/Number
  • 1
Journal Volume
  • 10
Ultima modifica
  • 2022-04-27
Resource Type
Dichiarazione dei diritti
License
DOI
ISSN
  • 2045-2322
Language

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